HAL will be down for maintenance from Friday, June 10 at 4pm through Monday, June 13 at 9am. More information
Skip to Main content Skip to Navigation
Journal articles

Quantum Corrections in Nanoplasmonics: Shape, Scale, and Material

Abstract : The classical treatment of plasmonics is insufficient at the nanometer-scale due to quantum mechanical surface phenomena. Here, an extension of the classical paradigm is reported which rigorously remedies this deficiency through the incorporation of first-principles surface response functions—the Feibelman d parameters—in general geometries. Several analytical results for the leading-order plasmonic quantum corrections are obtained in a first-principles setting; particularly, a clear separation of the roles of shape, scale, and material is established. The utility of the formalism is illustrated by the derivation of a modified sum rule for complementary structures, a rigorous reformulation of Kreibig's phenomenological damping prescription, and an account of the small-scale resonance shifting of simple and noble metal nanostructures.
Document type :
Journal articles
Complete list of metadata

Cited literature [47 references]  Display  Hide  Download

https://hal-iogs.archives-ouvertes.fr/hal-01549547
Contributor : Marie-Laure Edwards Connect in order to contact the contributor
Submitted on : Wednesday, June 28, 2017 - 6:09:28 PM
Last modification on : Friday, January 7, 2022 - 3:46:00 AM
Long-term archiving on: : Thursday, January 18, 2018 - 3:01:22 AM

File

PhysRevLett.118.157402.pdf
Publisher files allowed on an open archive

Identifiers

Citation

Thomas Christensen, Wei Yan, A.-P. Jauho, Marin Soljačić, N. Asger Mortensen. Quantum Corrections in Nanoplasmonics: Shape, Scale, and Material. Physical Review Letters, American Physical Society, 2017, 118, pp.57402. ⟨10.1103/PhysRevLett.118.157402⟩. ⟨hal-01549547⟩

Share

Metrics

Record views

86

Files downloads

127