Quantum Corrections in Nanoplasmonics: Shape, Scale, and Material - Archive ouverte HAL Access content directly
Journal Articles Physical Review Letters Year : 2017

Quantum Corrections in Nanoplasmonics: Shape, Scale, and Material

(1) , (2) , (3, 4) , (1) , (3, 5)
1
2
3
4
5

Abstract

The classical treatment of plasmonics is insufficient at the nanometer-scale due to quantum mechanical surface phenomena. Here, an extension of the classical paradigm is reported which rigorously remedies this deficiency through the incorporation of first-principles surface response functions—the Feibelman d parameters—in general geometries. Several analytical results for the leading-order plasmonic quantum corrections are obtained in a first-principles setting; particularly, a clear separation of the roles of shape, scale, and material is established. The utility of the formalism is illustrated by the derivation of a modified sum rule for complementary structures, a rigorous reformulation of Kreibig's phenomenological damping prescription, and an account of the small-scale resonance shifting of simple and noble metal nanostructures.
Fichier principal
Vignette du fichier
PhysRevLett.118.157402.pdf (567.94 Ko) Télécharger le fichier
Origin : Publisher files allowed on an open archive
Loading...

Dates and versions

hal-01549547 , version 1 (28-06-2017)

Identifiers

Cite

Thomas Christensen, Wei Yan, A.-P. Jauho, Marin Soljačić, N. Asger Mortensen. Quantum Corrections in Nanoplasmonics: Shape, Scale, and Material. Physical Review Letters, 2017, 118, pp.57402. ⟨10.1103/PhysRevLett.118.157402⟩. ⟨hal-01549547⟩
88 View
131 Download

Altmetric

Share

Gmail Facebook Twitter LinkedIn More