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Journal articles
Quantum Corrections in Nanoplasmonics: Shape, Scale, and Material
Abstract : The classical treatment of plasmonics is insufficient at the nanometer-scale due to quantum mechanical surface phenomena. Here, an extension of the classical paradigm is reported which rigorously remedies this deficiency through the incorporation of first-principles surface response functions—the Feibelman d parameters—in general geometries. Several analytical results for the leading-order plasmonic quantum corrections are obtained in a first-principles setting; particularly, a clear separation of the roles of shape, scale, and material is established. The utility of the formalism is illustrated by the derivation of a modified sum rule for complementary structures, a rigorous reformulation of Kreibig's phenomenological damping prescription, and an account of the small-scale resonance shifting of simple and noble metal nanostructures.
Cited literature [47 references]
https://hal-iogs.archives-ouvertes.fr/hal-01549547
Contributor : Marie-Laure Edwards <>
Submitted on : Wednesday, June 28, 2017 - 6:09:28 PM
Last modification on : Tuesday, August 6, 2019 - 11:38:23 AM
Long-term archiving on: : Thursday, January 18, 2018 - 3:01:22 AM
Contributor : Marie-Laure Edwards <>
Submitted on : Wednesday, June 28, 2017 - 6:09:28 PM
Last modification on : Tuesday, August 6, 2019 - 11:38:23 AM
Long-term archiving on: : Thursday, January 18, 2018 - 3:01:22 AM
File
PhysRevLett.118.157402.pdf
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